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In lean and near-stoichiometric flames, the larger N O formation rates are primarily the consequence of super-equilibrium concentrations of O and O H . Observed N O formation rates may be calculated using reactions (1H3), provided accurate values of the O and O H concentrations are used. In fuel-rich flames, super-equilibrium O and O H concentrations may account for some increase in the N O formation rate, but there is convincing experimental evidence that reactions between hydrocarbon species and molecular nitrogen play a significant role in the N O formation mechanism.
Roy. Soc. A 324, 201 (1971). 34. BARKER, M. , ROBERTS, A. G . and WRIGHT, S. J. Steam plant for the 1970's, Mechanical Engineering Convention, Institution of Mechanical Engineers, London (April 1969). 35. HOY, H . R. and ROBERTS, A. G . E. Meeting, San Francisco (Dec. 1971). 36. LONGWELL, J. P. and WEISS, N. A. Ind. Eng. , Ind. ) edn, 47, 1634(1955). International Symposium on Combustion, Rheinholt, New York (1956). International Symposium on Combustion, Butterworths, London (1959). p. 398. p. 664.
Removal of N O is assumed to occur by reaction with nitrogen-containing inter40 mediates to form molecular nitrogen. B o w m a n has shown that O atom concentrations can exceed partial equilibrium values in fuel-rich hydrocarbon combustion. However, the observed O atom concentrations still are not large enough to account for N O formation 38 CRAIG T. 7 - : — • l. 0 EQUIVALENCE RATIO FIG. 3. 0) in the flue gas of an oil-fired furnace with various amounts of pyridine added 41 to the fuel. FIG. 2.